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Kinetics and Mechanism of Oxidation of 1,3--Butylene Glycol by Dihydroxyditellutoargentate(III) in Alkaline Medium
2006
Journal:  
Turkish Journal of Chemistry
Author:  
Abstract:

The kinetics of oxidation of 1,3--butlene glycol (b - BG) by dihydroxyditelluto- argentate(III) were studied spectrophotometrically between 298.2 and 313.2 K in alkaline medium. The reaction rate showed pseudo-first order dependence in oxidant and fractional order in \ss-BG. The pseudo-first order rate constant kobs increased with an increase in the concentration of OH- and a decrease in the concentration of TeO42- . There was a negative salt effect and no free radicals were detected. Thus, the dihydroxymonotelluratoargentate(III) species is assumed to be the active species. The activation parameters along with the rate constants of the rate-determining step were calculated.

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Turkish Journal of Chemistry

Field :   Fen Bilimleri ve Matematik

Journal Type :   Uluslararası

Metrics
Article : 2.410
Cite : 1.692
2023 Impact : 0.068
Details
Turkish Journal of Chemistry